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I like Natalie and I like other Angel- names (Angelina, Angeline, Angie) but the two don't sound great together IMO. Something about the rhythm is off, and the end of Natalie blends into the beginning of Angelique. Also it clearly means "Christmas angel" which I find sappy, but that's probably not so obvious to non-name-nerds.
It's very CUTE, light, and would fit a Christmas baby.