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Callie definitely comes across as a diminutive. I don't think it stands alone.

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Cally/ie is sometimes short for Caroline, so I guess would work for Carolyn as well

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Or

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Calanthe
Calliope
Callista
Callisto
Calypso
Cara
Carla
Carlotta

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I think for a non Hindu to use Kali, it should definitely me a nickname or shortening of something else.

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http://www.behindthename.com/pnl/167578